https://doi.org/10.1007/s100510050950
Weak ferromagnetism in LaMnO3
1
Physics Department, Trinity College, Dublin 2, Ireland
2
Institut d'Électronique Fondamentale, Université Paris-Sud,
91405 Orsay Cedex, France
3
Laboratoire de Chimie des Solides, Université Paris-Sud,
91405 Orsay Cedex, France
Corresponding author: a fott@spec.saclay.cea.fr
Received:
8
January
1999
Published online: 15 October 1999
The magnetic properties of
crystals have been studied. The ac susceptibility
has been measured at frequencies ranging from 10 Hz to 1 000 Hz. The x = 0.25
crystal shows a typical ferromagnetic behaviour with a dimensionless SI
susceptibility of 6 below
limited by the
demagnetizing field. Both x = 0 and x = 0.06 crystals show very sharp
peaks in
and
at the Néel points, 139 K and 135 K respectively.
This is quite unlike the usual behaviour of an antiferromagnet.
Magnetization measurements on an untwinned single crystal of
show a weak moment of
at 4.2 K which is
directed along the c axis. The origin of this canted antiferromagnetic
structure is discussed in terms of anisotropy and of Dzyaloshinskii-Moriya
interaction. It is concluded that anistropy is insufficient to explain
the canted antiferromagnetism.
PACS: 75.25.+z – Spin arrangements in magnetically ordered materials (including neutron and spin-polarized electron studies, synchrotron-source X-ray scattering, etc.) / 75.50.Ee – Antiferromagnetics / 75.40.Gb – Dynamic properties (dynamic susceptibility, spin waves, spin diffusion, dynamic scaling, etc.)
© EDP Sciences, Società Italiana di Fisica, Springer-Verlag, 1999