https://doi.org/10.1007/s100510170337
Magnetic circular dichroism in Co 2p photoemission of Co/Cu(1 1 13): Separation of the fundamental spectra
1
Istituto Nazionale per la Fisica della Materia, TASC Laboratory,
34012 Trieste, Italy
2
Institut de Physique, Univ. Neuchâtel, 2001 Neuchâtel,
Switzerland
3
Magnetic Spectroscopy Group, Daresbury Laboratory, Warrington
WA4 4AD, UK
4
Laboratoire de Magnétisme Louis Néel, CNRS, 38043
Grenoble, France
5
ESRF, BP 220, 38043 Grenoble, France
Corresponding author: a panaccioneg@elettra.trieste.it
Received:
26
September
2000
Published online: 15 January 2001
We measured high-quality Co 2p magnetic circular dichroism (MCD) spectra
in photoemission for > 5 ML Co films grown on Cu(1 1 13) using a
"complete"experiment, where the sample magnetization and the light
helicity vector were reversed separately. We show how the four measured
spectra, MP
, can be used to make new linear combinations,
which correspond to the circular dichroism in the angular dependence
(CDAD), magnetic linear dichroism in the angular dependence (MLDAD) and MCD
spectra. The integrated signals of the MLDAD and CDAD can be used to
estimate the error caused by the difference in the degrees of magnetization
and light polarization, respectively, in the opposite alignments. The MCD
signal integrated over the entire 2p region does not average to zero, as
one would have expected from the sum rule for photoemission to a
non-interacting continuum state. There is a strong MCD signal in the entire
region between the
and
main lines with pronounced
satellite structure. The differences between the measured and calculated
results for an independent-particle and an atomic model indicate the
presence of interatomic electron correlation effects and configurational
mixing.
PACS: 75.30.Pd – Surface magnetism / 75.25.+z – Spin arrangements in magnetically ordered materials (including neutron and spin-polarized electron studies, synchrotron-source x-ray scattering, etc.) / 71.70.Ej – Spin-orbit coupling, Zeeman and Stark splitting, Jahn-Teller effect / 79.60.-i – Photoemission and photoelectron spectra
© EDP Sciences, Società Italiana di Fisica, Springer-Verlag, 2001