https://doi.org/10.1007/s10051-001-8701-6
Independent magnon states on magnetic polytopes
1
Universität Osnabrück, Fachbereich Physik,
Barbarastr. 7, 49069 Osnabrück, Germany
2
Universität Osnabrück, Fachbereich Physik,
Barbarastr. 7, 49069 Osnabrück, Germany
Institut für theoretische Physik,
Universität Magdeburg,
PO Box 4120, 39016 Magdeburg, Germany
Corresponding author: a jschnack@uos.de
Received:
27
August
2001
Revised:
18
October
2001
Published online: 15 December 2001
For many spin systems with constant isotropic antiferromagnetic next-neighbour Heisenberg coupling the minimal energies form a rotational band, i.e. depend approximately quadratically on the total spin quantum number S, a property which is also known as Landé interval rule. However, we find that for certain coupling topologies, including recently synthesised icosidodecahedral structures this rule is violated for high total spins. Instead the minimal energies are a linear function of total spin. This anomaly results in a corresponding jump of the magnetisation curve which otherwise would be a regular staircase.
PACS: 75.50.Xx – Molecular magnets / 75.10.Jm – Quantized spin models / 75.40.Cx – Static properties (order parameter, static susceptibility, heat capacities, critical exponents, etc.)
© EDP Sciences, Società Italiana di Fisica, Springer-Verlag, 2001