https://doi.org/10.1140/epjb/e2009-00306-1
Indications for the coexistence of closed orbit and quantum interferometer with the same cross section in the organic metal β′′-(ET)4(H3O)[ Fe(C2O4)3] .C6H4Cl2: persistence of Shubnikov-de Haas oscillations above 30 K
1
Laboratoire National des Champs Magnétiques Intenses (UPR 3228 CNRS, INSA, UJF, UPS) 143 avenue de Rangueil, 31400 Toulouse, France
2
Institució Catalana de Recerca i Estudis Avançats (ICREA), 08010 Barcelona, Spain
3
Institut de Ciència de Materials de Barcelona (ICMAB - CSIC), Campus UAB, 08193 Bellaterra, Catalunya, Spain
4
Institute of Problems of Chemical Physics, Russian Academy of Sciences, 142432 Chernogolovka, Moscow oblast, Russia
Corresponding author: a audouard@lncmp.org
Received:
20
April
2009
Revised:
24
June
2009
Published online:
11
September
2009
Shubnikov-de Haas (SdH) and de Haas-van Alphen (dHvA) oscillations spectra of the quasi-two dimensional charge transfer salt β′′-(ET)4(H3O)[ Fe(C2O4)3] .C6H4Cl2 have been investigated in pulsed magnetic fields up to 54 T. The data reveal three basic frequencies Fa, Fb and Fb - a, which can be interpreted on the basis of three compensated closed orbits at low temperature. However a very weak thermal damping of the Fourier component Fb, with the highest amplitude, is evidenced for SdH spectra above about 6 K. As a result, magnetoresistance oscillations are observed at temperatures higher than 30 K. This feature, which is not observed for dHvA oscillations, is in line with quantum interference, pointing to a Fermi surface reconstruction in this compound.
PACS: 71.18.+y – Fermi surface: calculations and measurements; effective mass, g factor / 71.20.Rv – Polymers and organic compounds / 72.15.Gd – Galvanomagnetic and other magnetotransport effects
© EDP Sciences, Società Italiana di Fisica, Springer-Verlag, 2009