https://doi.org/10.1140/epjb/e2014-40712-6
Regular Article
Ornstein-Zernike correlations and magnetic ordering in nanostructures
1
GES and GICM Groups, Instituto de Física-FCEN, Universidad de
Antioquia UdeA, Calle 70
No.
52-21, Medellín, Colombia
2
Grupo de Investigación en Modelamiento y Simulación Computacional,
Facultad de Ingenierías, Universidad de San Buenaventura Sec. Medellín,
A.A. 5222
Medellín,
Colombia
3
Departamento de Física, Universidad de Santiago de Chile (USACH);
CEDENNA, Santiago,
Chile
4
Facultad de Física, Pontificia Universidad Católica de Chile;
CEDENNA, Santiago,
Chile
a
e-mail: johanmazo@gmail.com
Received: 26 July 2013
Received in final form: 5 February 2014
Published online: 10 March 2014
In this paper we propose a Heisenberg variational approach to study pseudo-critical phenomena on ferromagnetic nanostructures. We combine a two-spin cluster 3-dimensional Heisenberg Hamiltonian with Orstein-Zernike correlations and consider several geometries and crystalline lattices to explore the relationship among these factors and the effective number of nearest neighbors defined in several kind of nanometric structures. With this method we examine the size at which the pseudo-critical temperature of a magnetic nanoparticle reaches its bulk value. Our results shed light on the nanoscopic-microscopic limit, evidencing in particular that when one dimension is very small, independently of how big the other dimensions become, it is not possible for the structure to reach the bulk-like behavior. The results of our model are in good agreement with experimental data and other available analytical models.
Key words: Solid State and Materials
© EDP Sciences, Società Italiana di Fisica and Springer-Verlag, 2014