https://doi.org/10.1140/epjb/e2015-60219-x
Regular Article
Generation of localized magnetic moments in the charge-density-wave state
1
Moscow Institute for Physics and Technology (State
University), 141700
Moscow,
Russia
2
Institute for Theoretical and Applied Electrodynamics, Russian
Academy of Sciences, 125412
Moscow,
Russia
3
All-Russia Research Institute of Automatics,
127055
Moscow,
Russia
a
e-mail: apexgreen57@gmail.com
Received: 18 March 2015
Received in final form: 4 June 2015
Published online: 3 August 2015
We propose a mechanism explaining the generation of localized magnetic moments in charge-density-wave compounds. Our model Hamiltonian describes an Anderson impurity placed in a host material exhibiting the charge-density wave. There is a region of the model’s parameter space, where even weak Coulomb repulsion on the impurity site is able to localize the magnetic moment on the impurity. The phase diagram of a single impurity at T = 0 is mapped. To establish the connection with experiment, the thermodynamic properties of a random impurity ensemble is studied. Magnetic susceptibility of the ensemble diverges at low temperature; heat capacity as a function of the magnetic field demonstrates pronounced low field peak. Both features are consistent with experiments on orthorhombic TaS3 and blue bronze.
Key words: Solid State and Materials
© EDP Sciences, Società Italiana di Fisica, Springer-Verlag, 2015